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Simultaneous CO

Jie ZHU,Wei WANG,Xiuning HUA,Zhou XIA,Zhou DENG

《环境科学与工程前沿（英文）》 2015年 第9卷 第6期   页码 1117-1129 doi: 10.1007/s11783-015-0812-z

摘要： The chemical looping concept provided a novel way to achieve carbon separation during the production of energy or substances. In this work, hydrogen generation with inherent CO capture in single packed bed reactor via this concept was discussed. Two oxygen carriers, Fe O 60 wt.% and Fe O 55 wt.%/CuO 5 wt.% supported by Al O , were made by ball milling method. First, according to the characteristics of the reduction breakthrough curve, a strict fuel supply strategy was selected to achieve simultaneous CO capture and H production. Then, in the long term tests using CO as fuel, it was proved that CuO addition improved hydrogen generation with the maximum intensity of 3700 μmol H ·g Fe O compared with Fe-Al of 2300 μmol H ·g Fe O . The overall CO capture efficiency remained 98%–98.8% over 100 cycles. Moreover, the reactivity of deactivated materials was recovered nearly like that of fresh ones by sintering treatment. Finally, two kinds of complex gases consist of CO, H , CH and CO were utilized as fuels to test the feasibility. The results showed all components could be completely converted by Fe-Cu-Al in the reduction stage. The intensity of hydrogen production and the overall CO capture efficiency were in the range of 2000–2400 μmol H ·g Fe O and 89%–95%, respectively.

关键词： CO2 capture     chemical looping hydrogen generation     iron based oxygen carriers     single packed bed reactor     long-term test     complex gases fuel    

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Systematical strategies for wastewater treatment and the generated wastes and greenhouse gases in China

Jingbo GUO, Fang MA, Yuanyuan QU, Ang LI, Liang WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 271-279 doi: 10.1007/s11783-011-0328-0

摘要： China now faces double challenges of water resources shortage and severe water pollution. To resolve Chinese water pollution problems and reduce its impacts on human health, economic growth and social development, the situation of wastewater treatment was investigated. Excess sludge and greenhouse gases (GHGs) emitted during wastewater treatment were also surveyed. It is concluded that Chinese water pollution problems should be systematically resolved with inclusion of wastewater and the solid waste and GHGs generated during wastewater treatment. Strategies proposed for the wastewater treatment in China herein were also adequate for other countries, especially for the developing countries with similar economic conditions to China.

关键词： wastewater treatment     solid waste     greenhouse gases     systematical strategies    

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Stability of an annular viscous liquid jet in compressible gases with different properties inside and

Chunji YAN, Maozhao XIE,

《能源前沿（英文）》 2010年 第4卷 第2期   页码 198-204 doi: 10.1007/s11708-009-0054-5

摘要： A spatial linear instability analysis is conducted on an annular viscous liquid jet injected into compressible gases and a three-dimensional model of the jet is developed. The model takes into account differences between the velocities, densities of the gases inside and outside of the liquid jet. Theoretical analysis reveals that there exist 9 dimensionless parameters controlling the instability of the liquid jet. Numerical computations reveal some basic characteristics in the breakup and atomization process of the liquid jet as well as influences of these relevant parameters. Major observations and findings of this study are as follows. The Mach number plays a destabilizing role and the inner Mach number has a greater effect on the jet instability than the outer Mach number. The Reynolds number always tends to promote the instabilities of the liquid jet, but its influence is very limited. The Weber number and the gas-to-liquid density ratio also have unstable effects and can improve the atomization of liquid jets. Furthermore, the effects of the Weber number and gas-to-liquid density ratio on the maximum growth rates of axisymmetric and non-axisymmetric disturbances and corresponding dominant wave numbers are manifested in a linear way, while that of the Mach number is non-linear. The effect of Reynolds on the maximum growth rates is non-linear, but the dominant wavenumber is almost not affected by the Reynolds number.

关键词： liquid jet     dominant wave number     compressibility     instability    

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analysis of using diethanolamine instead of methyldiethanolamine solution for GASCO’S Habshan acid gases

Samah Zaki NAJI, Ammar Ali ABD

《能源前沿（英文）》 2019年 第13卷 第2期   页码 317-324 doi: 10.1007/s11708-019-0622-2

摘要： Sweeting natural gas processes are mainly focused on removing carbon dioxide (CO ) and hydrogen sulfide (H S). The high-energy requirements and operational limitations make amine absorption process sensitive to any change in conditions. This paper presented a steady-state simulation using Hysys to reasonably predict removal amounts of carbon dioxide and hydrogen sulfide from natural gas with the diethanolamine (DEA) solvent. The product specifications are taken from the real plant (GASCO’S Habshan) which uses the methyldiethanolamine (MDEA) solvent, while this simulation uses DEA under the same operation conditions. First, the simulation validation has been checked with the data of the real plant. The results show accurate prediction for CO slippage and accepted agreement for H S content compared with the data of the plant. A parametric analysis has been performed to test all possible parameters that affect the performance of the acid gases removal plant. The effects of operational parameters are examined in terms of carbon dioxide and hydrogen sulfide contents in clean gas and reboiler duty.

关键词： acid gas     diethanolamine     methyldiethanolamine     carbon dioxide capturing     HYSYS simulation    

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Removal of multicomponent VOCs in off-gases from an oil refining wastewater treatment plant by a compost-based

Dan WU, Chunyan ZHANG, Li HAO, Changjun GENG, Xie QUAN,

《环境科学与工程前沿（英文）》 2009年 第3卷 第4期   页码 483-491 doi: 10.1007/s11783-009-0144-y

摘要： Waste gases from oil refining wastewater treatment plants are often characterized by the presence of multicomponent and various concentrations of compounds. An evaluation of the performance and feasibility of removing multicomponent volatile organic compounds (VOCs) in off-gases from oil refining wastewater treatment plants was conducted in a pilot-scale compost-based biofilter system. This system consists of two identical biofilters packed with compost and polyethylene (PE). This paper investigates the effects of various concentrations of nonmethane hydrocarbon (NMHC) and empty bed residence time (EBRT) on the removal efficiency of NMHC. Based on the experimental results and practical applications, an EBRT of 66 s was applied to the biofilter system. The removal efficiencies of NMHC were within the range of 47%―100%. At an EBRT of 66 s, the average removal efficiency of benzene, toluene, and xylene were more than 99%, 99%, and 100%, respectively. The results demonstrated that multicomponent VOCs in off-gases from the oil refining wastewater treatment plant could be successfully removed in the biofilter system, which may provide useful information concerning the design criteria and operation of full-scale biofilters.

关键词： biodegradation     volatile organic compounds (VOCs)     biofiltration     biofilter    

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GID complex regulates the differentiation of neural stem cells by destabilizing TET2

《医学前沿（英文）》 doi: 10.1007/s11684-023-1007-9

摘要： Brain development requires a delicate balance between self-renewal and differentiation in neural stem cells (NSC), which rely on the precise regulation of gene expression. Ten-eleven translocation 2 (TET2) modulates gene expression by the hydroxymethylation of 5-methylcytosine in DNA as an important epigenetic factor and participates in the neuronal differentiation. Yet, the regulation of TET2 in the process of neuronal differentiation remains unknown. Here, the protein level of TET2 was reduced by the ubiquitin-proteasome pathway during NSC differentiation, in contrast to mRNA level. We identified that TET2 physically interacts with the core subunits of the glucose-induced degradation-deficient (GID) ubiquitin ligase complex, an evolutionarily conserved ubiquitin ligase complex and is ubiquitinated by itself. The protein levels of GID complex subunits increased reciprocally with TET2 level upon NSC differentiation. The silencing of the core subunits of the GID complex, including WDR26 and ARMC8, attenuated the ubiquitination and degradation of TET2, increased the global 5-hydroxymethylcytosine levels, and promoted the differentiation of the NSC. TET2 level increased in the brain of the Wdr26+/− mice. Our results illustrated that the GID complex negatively regulates TET2 protein stability, further modulates NSC differentiation, and represents a novel regulatory mechanism involved in brain development.

关键词： TET2     GID complex     neural stem cells     differentiation of neurons    

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Combustion and emissions of RP-3 jet fuel and diesel fuel in a single-cylinder diesel engine

《能源前沿（英文）》 2023年 第17卷 第5期   页码 664-677 doi: 10.1007/s11708-021-0787-3

摘要： The combustion characteristics and emission behaviors of RP-3 jet fuel were studied and compared to commercial diesel fuel in a single-cylinder compression ignition (CI) engine. Engine operational parameters, including engine load (0.6, 0.7, and 0.8 MPa indicating the mean effective pressure (IMEP)), the exhaust gas recirculation (EGR) rate (0%, 10%, 20%, and 30%), and the fuel injection timing (−20, −15, −10, and −5 ° crank angle (CA) after top dead center (ATDC)) were adjusted to evaluate the engine performances of RP-3 jet fuel under changed operation conditions. In comparison to diesel fuel, RP-3 jet fuel shows a retarded heat release and lagged combustion phase, which is more obvious under heavy EGR rate conditions. In addition, the higher premixed combustion fraction of RP-3 jet fuel leads to a higher first-stage heat release peak than diesel fuel under all testing conditions. As a result, RP-3 jet fuel features a longer ignition delay (ID) time, a shorter combustion duration (CD), and an earlier CA50 than diesel fuel. The experimental results manifest that RP-3 jet fuel has a slightly lower indicated thermal efficiency (ITE) compared to diesel fuel, but the ITE difference becomes less noticeable under large EGR rate conditions. Compared with diesel fuel, the nitrogen oxides (NOx) emissions of RP-3 jet fuel are higher while its soot emissions are lower. The NOx emissions of RP-3 can be effectively reduced with the increased EGR rate and delayed injection timing.

关键词： RP-3 jet fuel     diesel     engine     combustion     emissions    

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The prior rules of designing Ti

Yingying Jian, Danyao Qu, Lihao Guo, Yujin Zhu, Chen Su, Huanran Feng, Guangjian Zhang, Jia Zhang, Weiwei Wu, Ming-Shui Yao

《化学科学与工程前沿（英文）》 2021年 第15卷 第3期   页码 505-517 doi: 10.1007/s11705-020-2013-y

摘要： Working temperature, sensitivity, and selectivity are some of the characteristics of the applied gas sensors. How to design and fabricate an ideal gas sensor working at room temperature is still challenging and attracting lots of interest. Two-dimensional (2D) materials with ultra-thin structure have been demonstrated as a family of ideal candidates to achieve this goal. Among them, Ti C T MXene, a kind of layered sheet synthesized by selectively etching MAX phases materials, shows remarkable potential to be the sensitive materials solely or in a composite. However, their designing rules are still lacking critical thinking from the viewpoint of the intrinsic property of Ti C T MXene based materials. In this article, two critical features, i.e., the thickness of the sensitive materials, and the scope of the analytes, are elaborated towards Ti C T MXene based gas sensors after characterizing the performance of sensing reducing gases (NH and CO) and oxidizing gas (NO ). First, the thinner the Ti C T MXene sensitive layer, the better the sensitivity. Second, the Ti C T MXene based gas sensor is not suitable for strong and moderate oxidation gas due to its ease of oxidation. These two rules are demonstrated, and could be considered with priority both in the future researches and practical applications.

关键词： MXene based sensor     prior     reducing gases     oxidizing gases    

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Impacts of methanol fuel on vehicular emissions: A review

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1553-4

摘要：

● Methanol effectively reduces CO, HC, CO2, PM, and PN emissions of gasoline vehicles.

关键词： Methanol fuel     Vehicular emission     Emission reduction     Cleaner fuel     Gasoline substitute    

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Calculations of narrow-band transimissities and the Planck mean absorption coefficients of real gases

Huaqiang CHU, Mingyan GU, Huaichun ZHOU, Fengshan LIU

《能源前沿（英文）》 2014年 第8卷 第1期   页码 41-48 doi: 10.1007/s11708-013-0292-4

摘要： Narrow-band transmissivities in the spectral range of 150 to 9300 cm and at a uniform resolution of 25 cm were calculated using the statistical narrow-band (SNB) model with the band parameters of Soufiani and Taine, the more recent parameters of André and Vaillon, and the line-by-line (LBL) method along with the HITEMP-2010 spectroscopic database. Calculations of narrow-band transmissivity were conducted for gas columns of different lengths and containing different isothermal and non-isothermal CO -H O-N mixtures at 1 atm. Narrow-band transmissivities calculated by the SNB model are in large relative error at many bands. The more recent SNB model parameters of André and Vaillon are more accurate than the earlier parameters of Soufiani and Taine. The Planck mean absorption coefficients of CO , H O, CO, and CH in the temperature range of 300 to 2500 K were calculated using the LBL method and different versions of the high resolution transmission (HITRAN) and high-temperature spectroscopic absorption parameters (HITEMP) spectroscopic databases. The SNB model was also used to calculate the Planck mean absorption coefficients of these four radiating gases. The LBL results of the Planck mean absorption coefficient were compared with the classical results of Tien and those from the SNB model.

关键词： transimissity     HITEMP     HITRAN     Planck mean absorption coefficients    

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Failure mode investigation of fuel cell for vehicle application

Zhongjun HOU, Renfang WANG, Keyong WANG, Weiyu SHI, Danming XING, Hongchun JIANG

《能源前沿（英文）》 2017年 第11卷 第3期   页码 318-325 doi: 10.1007/s11708-017-0488-0

摘要： The durability of proton exchange membrane fuel cells (PEMFCs) has been posing a key technical challenge to commercial spread of fuel cell vehicles (FCVs). To improve the durability, it is necessary to optimize the fuel cell system (FCS) design against failure modes. The fuel cell durability research method at FCS scale was exhibited, and the failure modes of fuel cell were experimentally investigated in this paper. It is found that the fuel cell dry operation, start/stop cycle and gas diffusion layer (GDL) flooding are typical failure modes of fuel cells. After the modifications against the failure modes, the durability of FCSs is improved to over 3000 h step by step.

关键词： proton exchange membrane fuel cell (PEMFC)     fuel cell system (FCS)     durability     failure mode     fuel cell vehicle (FCV)     carbon corrosion     water management    

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Numerical investigation of the effects of fuel spray type on the interaction of fuel spray and hot porous

ZHAO Zhiguo, XIE Maozhao

《能源前沿（英文）》 2008年 第2卷 第1期   页码 59-65 doi: 10.1007/s11708-008-0022-5

摘要： The interaction between two types of fuel spray and a hot porous medium is studied numerically by using an improved version of KIVA-3V code. The improved KIVA-3V code is incorporated with an impingement model, a heat transfer model and a linearized instability sheet atomization (LISA) model to model the hollow cone spray. An evaporating fuel spray impingement on a hot plane surface was simulated under conditions of experiments performed by Senda to validate the reasonability of the KIVA-3V code. The numerical results conform well with experimental data for spray radius in the liquid and the vapor phases. Computational results on the interaction of two types of the fuel spray and the hot porous medium show that the fuel spray can be split, which provides conditions for quick evaporation of fuel droplets and mixing of fuel vapor with air. The possibility of fuel droplets from hollow cone spray crossing the porous medium reduces compared with that from solid cone spray, with the same initial kinetic energy of fuel droplets in both injection types.

关键词： improved version     impingement     atomization     hollow     radius    

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Recent advances in cathode electrocatalysts for PEM fuel cells

Junliang ZHANG

《能源前沿（英文）》 2011年 第5卷 第2期   页码 137-148 doi: 10.1007/s11708-011-0153-y

摘要： Great progress has been made in the past two decades in the development of the electrocatalysts for proton exchange membrane fuel cells (PEMFCs). This review article is focused on recent advances made in the kinetic-activity improvement on platinum- (Pt-) based cathode electrocatalysts for the oxygen reduction reaction (ORR). The origin of the limited ORR activity of Pt catalysts is discussed, followed by a review on the development of Pt alloy catalysts, Pt monolayer catalysts, and shape- and facet-controlled Pt-alloy nanocrystal catalysts. Mechanistic understanding is reviewed as well on the factors contributing to the enhanced ORR activity of these catalysts. Finally, future directions for PEMFC catalyst research are proposed.

关键词： proton exchange membrane fuel cells (PEMFCs)     cathode electrocatalysts     platinum     oxygen reduction reaction (ORR)    

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TiO supported IrO for anode reversal tolerance in proton exchange membrane fuel cell

《能源前沿（英文）》 2022年 第16卷 第5期   页码 852-861 doi: 10.1007/s11708-021-0811-7

摘要： Fuel starvation can occur and cause damage to the cell when proton exchange membrane fuel cells operate under complex working conditions. In this case, carbon corrosion occurs. Oxygen evolution reaction (OER) catalysts can alleviate carbon corrosion by introducing water electrolysis at a lower potential at the anode in fuel shortage. The mixture of hydrogen oxidation reaction (HOR) and unsupported OER catalyst not only reduces the electrolysis efficiency, but also influences the initial performance of the fuel cell. Herein, Ti4O7 supported IrOx is synthesized by utilizing the surfactant-assistant method and serves as reversal tolerant components in the anode. When the cell reverse time is less than 100 min, the cell voltage of the MEA added with IrOx/Ti4O7 has almost no attenuation. Besides, the MEA has a longer reversal time (530 min) than IrOx (75 min), showing an excellent reversal tolerance. The results of electron microscopy spectroscopy show that IrOx particles have a good dispersity on the surface of Ti4O7 and IrOx/Ti4O7 particles are uniformly dispersed on the anode catalytic layer. After the stability test, the Ti4O7 support has little decay, demonstrating a high electrochemical stability. IrOx/Ti4O7 with a high dispersity has a great potential to the application on the reversal tolerance anode of the fuel cell.

关键词： proton exchange membrane fuel cell (PEMFC)     fuel starvation     cell reverse     reversal tolerance anode     oxygen evolution reaction    

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Footholds optimization for legged robots walking on complex terrain

《机械工程前沿（英文）》 2023年 第18卷 第2期 doi: 10.1007/s11465-022-0742-y

摘要： This paper proposes a novel continuous footholds optimization method for legged robots to expand their walking ability on complex terrains. The algorithm can efficiently run onboard and online by using terrain perception information to protect the robot against slipping or tripping on the edge of obstacles, and to improve its stability and safety when walking on complex terrain. By relying on the depth camera installed on the robot and obtaining the terrain heightmap, the algorithm converts the discrete grid heightmap into a continuous costmap. Then, it constructs an optimization function combined with the robot’s state information to select the next footholds and generate the motion trajectory to control the robot’s locomotion. Compared with most existing footholds selection algorithms that rely on discrete enumeration search, as far as we know, the proposed algorithm is the first to use a continuous optimization method. We successfully implemented the algorithm on a hexapod robot, and verified its feasibility in a walking experiment on a complex terrain.

关键词： footholds optimization     legged robot     complex terrain adapting     hexapod robot     locomotion control    

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标题 作者 时间 类型 操作

Simultaneous CO

Jie ZHU,Wei WANG,Xiuning HUA,Zhou XIA,Zhou DENG

期刊论文

Systematical strategies for wastewater treatment and the generated wastes and greenhouse gases in China

Jingbo GUO, Fang MA, Yuanyuan QU, Ang LI, Liang WANG

期刊论文

Stability of an annular viscous liquid jet in compressible gases with different properties inside and

Chunji YAN, Maozhao XIE,

期刊论文

analysis of using diethanolamine instead of methyldiethanolamine solution for GASCO’S Habshan acid gases

Samah Zaki NAJI, Ammar Ali ABD

期刊论文

Removal of multicomponent VOCs in off-gases from an oil refining wastewater treatment plant by a compost-based

Dan WU, Chunyan ZHANG, Li HAO, Changjun GENG, Xie QUAN,

期刊论文

GID complex regulates the differentiation of neural stem cells by destabilizing TET2

期刊论文

Combustion and emissions of RP-3 jet fuel and diesel fuel in a single-cylinder diesel engine

期刊论文

The prior rules of designing Ti

Yingying Jian, Danyao Qu, Lihao Guo, Yujin Zhu, Chen Su, Huanran Feng, Guangjian Zhang, Jia Zhang, Weiwei Wu, Ming-Shui Yao

期刊论文

Impacts of methanol fuel on vehicular emissions: A review

期刊论文

Calculations of narrow-band transimissities and the Planck mean absorption coefficients of real gases

Huaqiang CHU, Mingyan GU, Huaichun ZHOU, Fengshan LIU

期刊论文

Failure mode investigation of fuel cell for vehicle application

Zhongjun HOU, Renfang WANG, Keyong WANG, Weiyu SHI, Danming XING, Hongchun JIANG

期刊论文

Numerical investigation of the effects of fuel spray type on the interaction of fuel spray and hot porous

ZHAO Zhiguo, XIE Maozhao

期刊论文

Recent advances in cathode electrocatalysts for PEM fuel cells

Junliang ZHANG

期刊论文

TiO supported IrO for anode reversal tolerance in proton exchange membrane fuel cell

期刊论文

Footholds optimization for legged robots walking on complex terrain

期刊论文